By D. D. Eley, Herman Pines, Paul B. Weisz
(from preface)The assorted efforts of authors and the large scope of insurance undertaken in Advances in Catalysis—indeed, the breadth of catalysis itself—are good characterised by way of the seven chapters of this quantity. those chapters have been written by means of authors from departments of chemistry, chemical engineering, inorganic and analytical chemistry, fabrics technological know-how, and physics; from numerous universities; from significant commercial laboratories; and from a minimum of 3 institutes devoted in particular to catalysis!
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Additional info for Advances in Catalysis, Vol. 39
5. P. 25. Mercury intrusion curves at z, = 6, void radius distribution is the same as in Fig. 24. 5, and F, = 500 and lo00 A. 2 - 50 100 PRESSURE (ATMI 150 FIG. 26. 5. The void radius distribution is the same as in Fig. 24. 0 1 1 I I 1 1 30 40 50 60 70 PORE RADIUS 41 (pm) FIG. 27. Integral radius distributions of necks and voids, @(r) and F ( r ) [Eqs. (32) and (33)] calculated from mercury penetration and photomicrographic data, respectively. Curve 1 , the model of independent cylinders with a length proportional to their radii; curves 2 and 3 , Eq.
Relative activity as a function of time at various values of the deactivation rate constant. The time dependence of the critical radius is described by Eq. (50). P. ZHDANOV VI. Conclusion Modern percolation theory contains many interesting problems that usually are easily formulated. Solving these problems is customarily connected with extensive Monte Carlo simulations. However, the final results are often universal and can be employed in various fields of physics and chemistry. The data discussed in the present review reveal that applications of percolation theory have been particularly successful for describing the kinetic processes in porous solids, including desorption of condensate, mercury penetration, and catalytic deactivation by site coverage and pore blockage.
14 V . P . ZHDANOV 2. The mixed bond-site percolation problem yields a more complex way of constructing irregular lattices. In the framework of this problem, q b and q. (fractions of open bonds and sites of the original lattice) can have any values in the range from 0 to 1 simultaneously. If one analyzes, for example, the bond problem on an irregular lattice formed by blocking sites of the original regular lattice, the average coordination number for the irregular lattice is z = qszo, where zo is the coordination number for the original regular lattice.
Advances in Catalysis, Vol. 39 by D. D. Eley, Herman Pines, Paul B. Weisz